Unimolecular reactions are in principle the simplest chemical
reactions, because they only involve one molecule. The basic
mechanism, in which the competition between the chemical reaction
step and a collisional deactivation leads to a pressure-dependent
coefficient, has been understood for a long time. However, this is
a rapidly developing field, and many new and important discoveries
have been made in the past decade.
This First Part Part of Two CCK Volumes dealing with Unimolecular
Rections, deals with the Reaction Step. The first chapter is an
introduction to the whole project, aiming to cover the material
necessary to understand the content of the detailed chapters, as
well as the history of the development of the area. Chapter 2 is a
review of the modern view of the statistical theories, as embodied
in the various forms of RRKM theory. Chapter 3 deals with the fully
quantum mechanical view of reactive states as resonances.
. Presents considerable advances in the field made during the last
. Treats both the statistical as well as the fully quantum
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