In the present thesis we develop new strategies concerning the use
of lanthanide cations as spectroscopic probes for the study of
molecular structures in solution. A widespread interest for
lanthanides is mainly centered in two large fields: organic
synthesis and clinical practice. Systems containing lanthanides
enjoy a very favorable situation, since these ions feature high
coordination numbers, which assure rich binding chemistry, and at
the same time they possess the right spectroscopic properties to
monitor it. The present thesis develops the potentialities of
electronic spectroscopy of lanthanide systems in solution. We point
out and overcome the drawbacks which have mainly hampered this kind
of study so far, namely: a sensivity problem, an instrumental
problem and a calibration problem.
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